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Captured Nightmare was a Legendary Crafting Material in Diablo III before patch 2.0.6. It requires a Character Level of 1 to use, is account bound, and may be stacked up to 1000 times. It was required for the crafting of the Night's Reaping legendary mighty weapon. As of patch 2.0.6., it no longer drops, and existing Nightmares may be sold for 50,000 gold each.

The item had a chance to drop off the unique Enslaved Nightmares:

Enslaved nightmares were once human sorcerers who lost themselves to the dark arts. In fact, many still carry with them the shadow of the person they once were. If one listens carefully, their mournful cries can still be heard.

Diablo III Crafting Materials

Regular Salvaged and Dropped Materials